Stability and electronic properties of bilayer graphene spirals

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Date

2021-01-19T00:00:00

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Publisher

Elsevier B.V.

Abstract

Spiral topology offers many potential applications to next-generation nanoelectronic devices. The ab-initio simulations are used to investigate the stability and electronic properties of the hexagonal and triangular double-layer spiral (DLS). A room temperature molecular dynamics (MD) simulation reveals that the AA stacking of triangular DLS (t-DLS) is thermodynamically stable, however, the AA stacking of hexagonal DLS (h-DLS)is found to get distorted. When h-DLS and t-DLS are subjected to tensile strain the h-DLS behaved elastically, however, the t-DLS is extremely brittle. Both h-DLS and t-DLS are observed to be metallic in an equilibrium state. On applying an electric field, the h-DLS remains metallic, whereas, the t-DLS becomes a semiconductor. The bandgap of t-DLS is observed to open up even for a small magnitude of electric field. Furthermore, we also found that the triangular-shaped bilayer spiral topology gives rise to an intrinsic Rashba splitting. Our study opens up new and innovative ideas for investigating the spiral-shaped nano-structures. � 2021 Elsevier B.V.

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Keywords

Band-splitting, Electronic properties, Graphene spirals, Rashba-splitting, Thermodynamical stability

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